CHEM623 (Chemometrics)

Syllabus for Spring 2009

Texts & Resources Catalog Description Course Requirements
Grading Calendar General Course information
Prof. Steven Brown
Office: 239 Brown Laboratory   Office Hours: T,W 10-11, R 9-10
Voice mail: 831-6861 
E-mail: sdb@udel.edu
Spring 2009 
9:05-9:55 MWF  
116 BrL
Texts & Resources
Texts/Resources/Readings/Supplies

Required Text:

There is no single suitable text for this subject and no text is required.
There will be readings from handouts and papers from the literature available for download at the Chem 623 site on Sakai. You will need to be registered for the course as a student or as a listener to gain access to the Sakai site.

Other Required Items:

1. Ready access to a suitable computer where you can install and use Matlab data analysis software. This can be a group computer or your own computer. You will need access to a printer and the internet from this computer.

2. Matlab computational software installed and functional on your computer. You can use Matlab at some campus computing sites, get access to your group's Matlab software or get Matlab software for campus use only from Pat McMahon. If you don't have easy, constant access to a recent version of this software, you will need to purchase a student version directly from Mathworks. An older version of Matlab will probably not work with some of the chemometrics software provided. If you purchase a student version, be sure to get it directly from Mathworks to avoid getting an out-of-date installation.

If you already know a suitable data analysis language, you may use it in this course; doing work in R, Igor, or Mathematica software is acceptable for homework and exams. You will need to port the chemometrics software that I provide you in Matlab or find a suitable replacement chemometrics package in your language of choice. Please note that Excel/Visual Basic is not an acceptable language for work in this course.

3. Software from Chem 623 for use in the Matlab computational environment. This semester, we will use the last public-domain version (v1.3) of the PLS Toolbox for demonstrations, and you can use it on homework and for the exams. This Matlab-based software is free for you to use in the course and beyond, but there is no support available from Eigenvector, the company that now sells the Toolbox. You must be enrolled in the course to get the chemometrics software.

Materials to be used during the course include: simulations, short video clips and analysis of some datasets using software provided and software available from the internet. You will need to dowload data sets and software packages and to check some work against published results available on the internet. You will be asked to submit your work in digital form (as a Word or PDF file) via Sakai because of the length of the homework sets and exams. You will need to become proficient at plotting and summarizing results of analyses.

Learning Resources:
Full lecture notes will be available in PDF format online, through Sakai. I will also provide PDF or hardcopy of supporting material. You are expected to attend lecture and to read material that I provide. I am unable to provide full transcripts for all demonstrations and video clips shown in the course.
 
Student feedback on instruction:
I will ask for student feedback at midterm for course/instructor improvement purposes. There will also be an end-of-term student evaluation with a supplement to departmental student evaluation form.
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Catalog Description

Chemistry 623 is a graduate-level, overview course in the analysis of data generated from instrumentation used in chemistry, biochemistry and related fields. The emphasis is on the understanding and practical application of chemometric methods. The course is intended for graduate students or for advanced majors in chemistry, biochemistry or chemical engineering who need to analyze data obtained from such instruments. This course presumes some knowledge of basic statistics and some prior exposure to simple computational computer programming. Brief reviews of concepts from probability, decision theory and experimental designs are provided to provide background, as is a discussion of processing of chemical signals to improve signal quality. The course's main focus is on the systematic evaluation of high-dimensional data through multivariate calibration and classification of multivariate chemical responses.

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Course Requirements and Policies

Course Requirements

This course is an introduction to computational analysis of data from chemical instrumentation. Chemometrics involves some math, so you will need to become comfortable with probability, statistic tests, matrix algebra and regression. You will learn a mixture of theory and practice, and will be asked to implement the theory in working computer code. Much of the code will be made available to you, but you will need to know how to make changes to existing code to do some of the work required. This skill will enable you to make use of the large code base available on the web.
 
Each homework set will involve some theory, some computation and some critcal evaluation of results.
 
Course Policies

Academic Honesty:

You are encouaged to become familiar with The University’s Policy of Academic Honesty found in the UD Student Guide to University Policies. More on the whole issue of academic integrity can be found here. Policies delineated in the Guide apply to this course. While homework sets for Chem 623 can be done in collaboration with others enrolled in the course, all work on the out-of-class examinations must be done entirely independently. By turning work into the instructor of this course, you acknowledge being made aware of the academic honesty policy and affirm your adherence to the letter and spirit of the policy.

Assignments:

Homework deadlines are posted and you are expected to meet the deadlines. If you have a problem and cannot make the deadline, please let me know. I may be able to allow some extra time for a once-only problem. Repeated late work will be penalized. Work missed for a reason (illness, conference travel, etc.) can be made up without penalty.

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Grading

Grading, Evaluation Policies and Procedures:

The course will be marked on the basis of your performance on homework, on a 3-day take-home midterm exam and on a 5 day, take-home, calculation-based final exam. The grade given will be determined on the basis of the total number of points earned.

The distribution of points is as follows:

Task                                                        Points

Homework (5 sets, each worth 20 pts): 100 pts
MidTerm Exam (4/6-4/9/09):                   50 pts
Final Examination(5/21-5/26/09):           100 pts

TOTAL:                                                 250 pts



Grading Scale:

    > 200 pts   A
151-199 pts   B
101-150 pts   C
 50 -100 pts   D
     < 50 pts    F

The average grade earned by students in this course has been B+

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Calendar

Tentative Schedule for Lectures:

All lectures are scheduled for 0905-0955 MWF in 116 Brown Laboratory.
This schedule is approximate and may vary to reflect scheduling changes and student needs.

Week      Topics to be Covered

2/9/09    Overview of Chemometrics, Introduction to Random Variables

2/16/09  Estimation, Confidence Intervals and Statistical Testing

2/23/09  Linear Regression Methods

3/2/09    Experimental Design

3/9/09    Signal Processing Methods

3/16/09  Pattern Recognition Methods -1- Exploratory Analysis

3/23/09  Pattern Recognition Methods -2- Supervised Methods

3/30/09  SPRING BREAK

4/6/09    Pattern Recognition Methods - 3- Advanced Methods
             MIDTERM EXAM 4/6-4/9/09 (Take Home, Computer-Based)

4/13/09  Chemical Calibration - 1 - Curve Fitting Data

4/20/07  Chemical Calibration - 2- Classical and Inverse Analysis

4/27/07  Chemical Calibration - 3- Soft Calibration

5/4/07    Chemical Calibration - 4- More on PLS Regression

5/11/07  Chemical Calibration - 5- Multiway and Nonlinear Calibration Methods

5/18/07  Self-Modeling Methods in Evolving Systems

5/20-26/07  FINAL EXAMINATION (Take Home, Computer-Based)

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General course information

Course information

Course pre-requisites:

This course presumes some knowledge of chemical instrumentation at the level of Chem 437 and Chem 438. Students should also have had an exposure to basic statistics as covered in an elementary statistics course or in Chem 120. Prior experience with scientific programming is not required but helpful.

Course Description:

This course covers an introduction to analysis of data from chemical instrumentation.

A brief review of basic statistics and probability is given, then the partitioning of data by variance is demonstrated. Regression methods are introduced to model the sources of variance, and approaches are covered to develop, evaluate and improve regression models.Soft modeling is developed as a way to deal with bias created from model-data mismatches, and soft modeling-based projections are shown effective at visual examination of multivariate data such as spectra.Methods are then presented top relate multivariate data to group and to external properties. Prediction of group membership is demonstrated, and prediction of external property is discussed in some detail. As a final topic, methods for discovery of underlying chemical signatures of the pure components comprising a mixed response is discussed and methods for systematic discovery of those components are presented

Course Objectives:

Students completing this course should be able to read, understandand critically evaluate literature making use of basic chemometrics techniques. They should also be able to perform basic chemometrics by developing MATLAB code or by modifying code provided by others.

Completion of this course will provide the student a foundation for research in chemometrics or for applying chemometric methods in other research projects.

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Last Updated: 11 February 2009

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